Deposition of 236U from atmospheric nuclear testing in Washington state (USA) and the Pechora region (Russian Arctic)

Michael E. Ketterer, Aran D. Groves, Brian J. Strick, Craig S. Asplund, Vivienne J. Jones

Research output: Contribution to journalArticlepeer-review

19 Scopus citations

Abstract

Stratospheric fallout-derived 236U has been detected by sector field ICPMS at two field locations for which our laboratory possessed available archived samples: A) four soil cores from Washington state (northwestern USA) and B) sediment cores from three small lakes in the Pechora region (Russian Arctic). Four Washington state soil cores exhibit 236U inventories of 8.1 ± 1.3, 11.1 ± 0.9, 18 ± 2, and 30.2 ± 3.9 Tatoms/m2; the respective 239Pu contents are 52.9 ± 3.5, 67 ± 3, 71 ± 2, and 151 ± 2 Tatoms/m2. A 236U/239Pu atom ratio of 0.19 ± 0.04 (1 SD) has been determined from the Washington state soil cores. The three Pechora region lake cores each exhibit coincident maxima in their 236U and 239Pu atom concentration profiles. The 236U/238U atom ratios are controlled by two independent factors; 236U is from fallout deposition and 238U concentrations are a property of the geochemical distribution of naturally occurring U. A 236U/238U atom ratio as high as 8.9 × 10-6 has been observed for acid-leached soils containing Pu solely derived from bomb-test fallout. Accordingly, a non-zero 236U background from stratospheric fallout must be recognized and taken into account when detectable 236U is used to infer specific local or regional influences of reactor-irradiated U.

Original languageEnglish (US)
Pages (from-to)143-149
Number of pages7
JournalJournal of Environmental Radioactivity
Volume118
DOIs
StatePublished - Apr 1 2013

Keywords

  • Atmospheric nuclear testing
  • Plutonium isotopes
  • U
  • Uranium isotopes

ASJC Scopus subject areas

  • Environmental Chemistry
  • Waste Management and Disposal
  • Pollution
  • Health, Toxicology and Mutagenesis

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